We propose a driven optical cavity quantum electrodynamics (QED) setup aimed at directly probing energy transport dynamics in photosynthetic biomolecules. We show that detailed information concerning energy transfer paths and delocalization of exciton states can be inferred (and exciton energies estimated) from the statistical properties of the emitted photons. This approach provides us with a spectroscopic tool to interrogate biological systems in terms of quantum optical phenomena which have usually been studied in solid-state or atomic systems (e.g., semiconductor quantum dots and trapped atoms) and which are now extended to a broader range of spectroscopy experiments.

Probing biological light-harvesting phenomena by optical cavities / F. Caruso;S. K. Saikin;E. Solano;S. F. Huelga;A. Aspuru-Guzik;M. B. Plenio. - In: PHYSICAL REVIEW. B, CONDENSED MATTER AND MATERIALS PHYSICS. - ISSN 1098-0121. - ELETTRONICO. - 85:(2012), pp. 125424-1-125424-10. [10.1103/PhysRevB.85.125424]

Probing biological light-harvesting phenomena by optical cavities

CARUSO, FILIPPO;
2012

Abstract

We propose a driven optical cavity quantum electrodynamics (QED) setup aimed at directly probing energy transport dynamics in photosynthetic biomolecules. We show that detailed information concerning energy transfer paths and delocalization of exciton states can be inferred (and exciton energies estimated) from the statistical properties of the emitted photons. This approach provides us with a spectroscopic tool to interrogate biological systems in terms of quantum optical phenomena which have usually been studied in solid-state or atomic systems (e.g., semiconductor quantum dots and trapped atoms) and which are now extended to a broader range of spectroscopy experiments.
2012
85
125424-1
125424-10
F. Caruso;S. K. Saikin;E. Solano;S. F. Huelga;A. Aspuru-Guzik;M. B. Plenio
File in questo prodotto:
File Dimensione Formato  
PhysRevB.85.125424.pdf

Accesso chiuso

Tipologia: Pdf editoriale (Version of record)
Licenza: Tutti i diritti riservati
Dimensione 1.86 MB
Formato Adobe PDF
1.86 MB Adobe PDF   Richiedi una copia

I documenti in FLORE sono protetti da copyright e tutti i diritti sono riservati, salvo diversa indicazione.

Utilizza questo identificatore per citare o creare un link a questa risorsa: https://hdl.handle.net/2158/849966
Citazioni
  • ???jsp.display-item.citation.pmc??? ND
  • Scopus 28
  • ???jsp.display-item.citation.isi??? 28
social impact