Molecular approaches for the optimization of electron spin-based quantum bits and quantum logic gates

This work highlights the different possibilities given by a rational chemical approach to obtain molecular-based quantum bits and quantum logic gates as an appealing and alternative platform for implementing quantum computation. This work resumes the three years of the author's work on this subject, mainly presenting and focusing on experimental results obtained for some new potential hydrogen-free molecular qubits, multi-qubit structures, and state-of-the-art EPR-based (Electron Paramagnetic Resonance) experiments on an archetypical vanadyl-based qubit.